Chemical asymmetric synthesis | Nature

Chemical asymmetric synthesis | Nature

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ABSTRACT Thalidomide comes in two forms: a left-handed compound which is a powerful tranquilizer, and a right-handed version which can disrupt fetal development causing severe handicap. As a necessary consequence of synthetic methods available in the early 1960s the two forms were present in equal proportions in the manufactured drug, with catastrophic consequences. The thalidomide story is perhaps the most painful reminder of the importance of stereochemistry—the spatial ordering of groups in a molecule can be as influential as the chemical nature of the groups themselves. A principal problem in organic synthesis is, therefore, the development of methods for producing complex molecules with a stereochemically defined structure. Access through your institution Buy or subscribe This is a preview of subscription content, access via your institution ACCESS OPTIONS Access through your institution Subscribe to this journal Receive 51 print issues and online access $199.00 per year only $3.90 per issue Learn more Buy this article * Purchase on SpringerLink * Instant access to full article PDF Buy now Prices may be subject to local taxes which are calculated during checkout ADDITIONAL ACCESS OPTIONS: * Log in * Learn about institutional subscriptions * Read our FAQs * Contact customer support SIMILAR CONTENT BEING VIEWED BY OTHERS CATALYTIC ASYMMETRIC SYNTHESIS OF _META_ BENZENE ISOSTERES Article 21 August 2024 CHEMICAL SYNTHESIS AS A DISCOVERY PLATFORM IN IMMUNOSUPPRESSION AND DETERMINATION OF MODE OF ACTION Article 04 January 2024 MODULAR, AUTOMATED SYNTHESIS OF SPIROCYCLIC TETRAHYDRONAPHTHYRIDINES FROM PRIMARY ALKYLAMINES Article Open access 04 October 2023 REFERENCES * Pratt, A. J., Davies, S. G., Brown, J. M. & Fleet, G. W. J. _Chemy Br._ 25, 259–268 (1989). Google Scholar  * Morrison, J. D. (ed.) _Asymmetric Synthesis_ Vol 1–5 (Wiley, New York, 1983–5). * Brunner, H. _Topics Stereochem._ 18, 129–248 (1988). CAS  Google Scholar  * Jacques, J., Wilen, S. H. & Collet, A. _Enantiomers, Racemates and Resolutions_ (Wiley, New York, 1981). Google Scholar  * Evans, D. A., Chapman, K. T. & Bisaha, J. _J. Am. chem. Soc._ 110, 1238–1256 (1988). Article  CAS  Google Scholar  * Gao, Y. _et al._ _J. Am. chem. Soc._ 109, 5765–5777 (1987). Article  CAS  Google Scholar  * Fleet, G. W. J., Ransden, N. G. & Witty, D. R. _Tetrahedron_ 45, 327–336 (1989). Article  CAS  Google Scholar  * Davies, S. G. _et al._ _Phil. Trans. R. Soc._ A326, 619–631 (1988). Article  ADS  CAS  Google Scholar  * Davies, S. G. _Pure appl. Chem._ 60, 13–20 (1988). Article  CAS  Google Scholar  * Davies, S. G. _et al._ _Bull. Soc. chim. Fr._ 608–630 (1987). * Bashiardes, G. & Davies, S. G. _Tetrahedron Lett._ 28, 5563–5564 (1987). Article  CAS  Google Scholar  * Brown, S. L., Davies, S. G., Foster, D. F., Seeman, J. I. & Warner, P. _Tetrahedron Lett._ 27, 623–626 (1986). Article  CAS  Google Scholar  * Porter, R. & Clark, S. (eds) _Enzymes in Organic Synthesis, Ciba Foundation Symp. 111_ (Pitman, London, 1985). * Schneider, M. P. (ed.) _Enzymes as Catalysts in Organic Synthesis_ (Riedel, Dordrecht, 1986). Google Scholar  * Jones, J. B. _Tetrahedron_ 42, 3351–3400 (1986). Article  CAS  Google Scholar  * Yamada, H. & Shimizu, S. _Angew. Chem. Int. Edn Engl._ 27, 622–640 (1988). Article  Google Scholar  * Pratt, A. J. _Chemy Br._ 25, 282–287 (1989). CAS  Google Scholar  * Bednarski, M. D. _et al._ _J. Am. chem. Soc._ 111, 627–635 (1989). Article  CAS  Google Scholar  * Kagan, H. B. _Comprehensive Organometallic Chemistry_ Vol. 8, 560–600 (eds Wilkinson, G., Stone, F. G. A. & Abel, E. W.) (Pergamon, Oxford, 1982). Google Scholar  * Brown, J. M. & Chaloner, P. _Catalysis with Metal-Phosphine Complexes_ Ch. 4, 131–170 (ed. Pignolet, L.) (Plenum, New York, 1984). Google Scholar  * James, B. R. _Comprehensive Organometallic Chemistry_ Vol. 8, Ch. 51 (eds Wilkinson, G., Stone, F. G. A. & Abel, E. W.) (Pergamon, Oxford, 1982). Google Scholar  * Takaya, H. _et al._ _J. Am. chem. Soc._ 109, 1596–1598 (1987). Article  CAS  Google Scholar  * Kitamura, M. _et al._ _J. Am. chem. Soc._ 110, 629–631 (1988). Article  CAS  Google Scholar  * Kagan, H. B. & Fiaud, J.-C. _Topics Stereochem._ 18, 249–330 (1988). CAS  Google Scholar  * Brown, J. M., Cutting, I. & James, A. P. _Bull. Soc. chim. Fr._ 212–219 (1988). * Brown, J. M. _Angew. Chem., Int. Edn Engl._ 26, 191–204 (1987). Google Scholar  * Oguni, N. & Omi, T. _Tetrahedron Lett._ 25, 2823–2827 (1984). Article  CAS  Google Scholar  * Kitamura, M., Suga, S., Kawai, K. & Noyori, R. _J. Am. chem. Soc._ 108, 6071–6072 (1986). Article  CAS  Google Scholar  * Soai, K., Ookawa, A., Kaba, T. & Ogawa, K. _J. Am. chem. Soc._ 109, 7111–7119 (1987). Article  CAS  Google Scholar  * Noyori, R., Suga, S., Kawai, K., Okada, S. & Kitamura, M. _Pure appl. Chem._ 60, 1597–1612 (1988). Article  CAS  Google Scholar  * Oguni, N., Matsuda, Y. & Kaneko, T. _J. Am. chem. Soc._ 110, 7877–7879 (1988). Article  CAS  Google Scholar  * Kitamura, A., Okada, S., Suga, S. & Noyori, R. _J. Am chem. Soc._ 111, 4028–4036 (1989). Article  CAS  Google Scholar  Download references AUTHOR INFORMATION AUTHORS AND AFFILIATIONS * Dyson Perrins Laboratory, South Parks Road, Oxford, OX1 3QY, UK John M. Brown & Stephen G. Davies Authors * John M. Brown View author publications You can also search for this author inPubMed Google Scholar * Stephen G. Davies View author publications You can also search for this author inPubMed Google Scholar RIGHTS AND PERMISSIONS Reprints and permissions ABOUT THIS ARTICLE CITE THIS ARTICLE Brown, J., Davies, S. Chemical asymmetric synthesis. _Nature_ 342, 631–636 (1989). https://doi.org/10.1038/342631a0 Download citation * Issue Date: 07 December 1989 * DOI: https://doi.org/10.1038/342631a0 SHARE THIS ARTICLE Anyone you share the following link with will be able to read this content: Get shareable link Sorry, a shareable link is not currently available for this article. Copy to clipboard Provided by the Springer Nature SharedIt content-sharing initiative

ABSTRACT Thalidomide comes in two forms: a left-handed compound which is a powerful tranquilizer, and a right-handed version which can disrupt fetal development causing severe handicap. As a


necessary consequence of synthetic methods available in the early 1960s the two forms were present in equal proportions in the manufactured drug, with catastrophic consequences. The


thalidomide story is perhaps the most painful reminder of the importance of stereochemistry—the spatial ordering of groups in a molecule can be as influential as the chemical nature of the


groups themselves. A principal problem in organic synthesis is, therefore, the development of methods for producing complex molecules with a stereochemically defined structure. Access


through your institution Buy or subscribe This is a preview of subscription content, access via your institution ACCESS OPTIONS Access through your institution Subscribe to this journal


Receive 51 print issues and online access $199.00 per year only $3.90 per issue Learn more Buy this article * Purchase on SpringerLink * Instant access to full article PDF Buy now Prices may


be subject to local taxes which are calculated during checkout ADDITIONAL ACCESS OPTIONS: * Log in * Learn about institutional subscriptions * Read our FAQs * Contact customer support


SIMILAR CONTENT BEING VIEWED BY OTHERS CATALYTIC ASYMMETRIC SYNTHESIS OF _META_ BENZENE ISOSTERES Article 21 August 2024 CHEMICAL SYNTHESIS AS A DISCOVERY PLATFORM IN IMMUNOSUPPRESSION AND


DETERMINATION OF MODE OF ACTION Article 04 January 2024 MODULAR, AUTOMATED SYNTHESIS OF SPIROCYCLIC TETRAHYDRONAPHTHYRIDINES FROM PRIMARY ALKYLAMINES Article Open access 04 October 2023


REFERENCES * Pratt, A. J., Davies, S. G., Brown, J. M. & Fleet, G. W. J. _Chemy Br._ 25, 259–268 (1989). Google Scholar  * Morrison, J. D. (ed.) _Asymmetric Synthesis_ Vol 1–5 (Wiley,


New York, 1983–5). * Brunner, H. _Topics Stereochem._ 18, 129–248 (1988). CAS  Google Scholar  * Jacques, J., Wilen, S. H. & Collet, A. _Enantiomers, Racemates and Resolutions_ (Wiley,


New York, 1981). Google Scholar  * Evans, D. A., Chapman, K. T. & Bisaha, J. _J. Am. chem. Soc._ 110, 1238–1256 (1988). Article  CAS  Google Scholar  * Gao, Y. _et al._ _J. Am. chem.


Soc._ 109, 5765–5777 (1987). Article  CAS  Google Scholar  * Fleet, G. W. J., Ransden, N. G. & Witty, D. R. _Tetrahedron_ 45, 327–336 (1989). Article  CAS  Google Scholar  * Davies, S.


G. _et al._ _Phil. Trans. R. Soc._ A326, 619–631 (1988). Article  ADS  CAS  Google Scholar  * Davies, S. G. _Pure appl. Chem._ 60, 13–20 (1988). Article  CAS  Google Scholar  * Davies, S. G.


_et al._ _Bull. Soc. chim. Fr._ 608–630 (1987). * Bashiardes, G. & Davies, S. G. _Tetrahedron Lett._ 28, 5563–5564 (1987). Article  CAS  Google Scholar  * Brown, S. L., Davies, S. G.,


Foster, D. F., Seeman, J. I. & Warner, P. _Tetrahedron Lett._ 27, 623–626 (1986). Article  CAS  Google Scholar  * Porter, R. & Clark, S. (eds) _Enzymes in Organic Synthesis, Ciba


Foundation Symp. 111_ (Pitman, London, 1985). * Schneider, M. P. (ed.) _Enzymes as Catalysts in Organic Synthesis_ (Riedel, Dordrecht, 1986). Google Scholar  * Jones, J. B. _Tetrahedron_ 42,


3351–3400 (1986). Article  CAS  Google Scholar  * Yamada, H. & Shimizu, S. _Angew. Chem. Int. Edn Engl._ 27, 622–640 (1988). Article  Google Scholar  * Pratt, A. J. _Chemy Br._ 25,


282–287 (1989). CAS  Google Scholar  * Bednarski, M. D. _et al._ _J. Am. chem. Soc._ 111, 627–635 (1989). Article  CAS  Google Scholar  * Kagan, H. B. _Comprehensive Organometallic


Chemistry_ Vol. 8, 560–600 (eds Wilkinson, G., Stone, F. G. A. & Abel, E. W.) (Pergamon, Oxford, 1982). Google Scholar  * Brown, J. M. & Chaloner, P. _Catalysis with Metal-Phosphine


Complexes_ Ch. 4, 131–170 (ed. Pignolet, L.) (Plenum, New York, 1984). Google Scholar  * James, B. R. _Comprehensive Organometallic Chemistry_ Vol. 8, Ch. 51 (eds Wilkinson, G., Stone, F. G.


A. & Abel, E. W.) (Pergamon, Oxford, 1982). Google Scholar  * Takaya, H. _et al._ _J. Am. chem. Soc._ 109, 1596–1598 (1987). Article  CAS  Google Scholar  * Kitamura, M. _et al._ _J.


Am. chem. Soc._ 110, 629–631 (1988). Article  CAS  Google Scholar  * Kagan, H. B. & Fiaud, J.-C. _Topics Stereochem._ 18, 249–330 (1988). CAS  Google Scholar  * Brown, J. M., Cutting, I.


& James, A. P. _Bull. Soc. chim. Fr._ 212–219 (1988). * Brown, J. M. _Angew. Chem., Int. Edn Engl._ 26, 191–204 (1987). Google Scholar  * Oguni, N. & Omi, T. _Tetrahedron Lett._ 25,


2823–2827 (1984). Article  CAS  Google Scholar  * Kitamura, M., Suga, S., Kawai, K. & Noyori, R. _J. Am. chem. Soc._ 108, 6071–6072 (1986). Article  CAS  Google Scholar  * Soai, K.,


Ookawa, A., Kaba, T. & Ogawa, K. _J. Am. chem. Soc._ 109, 7111–7119 (1987). Article  CAS  Google Scholar  * Noyori, R., Suga, S., Kawai, K., Okada, S. & Kitamura, M. _Pure appl.


Chem._ 60, 1597–1612 (1988). Article  CAS  Google Scholar  * Oguni, N., Matsuda, Y. & Kaneko, T. _J. Am. chem. Soc._ 110, 7877–7879 (1988). Article  CAS  Google Scholar  * Kitamura, A.,


Okada, S., Suga, S. & Noyori, R. _J. Am chem. Soc._ 111, 4028–4036 (1989). Article  CAS  Google Scholar  Download references AUTHOR INFORMATION AUTHORS AND AFFILIATIONS * Dyson Perrins


Laboratory, South Parks Road, Oxford, OX1 3QY, UK John M. Brown & Stephen G. Davies Authors * John M. Brown View author publications You can also search for this author inPubMed Google


Scholar * Stephen G. Davies View author publications You can also search for this author inPubMed Google Scholar RIGHTS AND PERMISSIONS Reprints and permissions ABOUT THIS ARTICLE CITE THIS


ARTICLE Brown, J., Davies, S. Chemical asymmetric synthesis. _Nature_ 342, 631–636 (1989). https://doi.org/10.1038/342631a0 Download citation * Issue Date: 07 December 1989 * DOI:


https://doi.org/10.1038/342631a0 SHARE THIS ARTICLE Anyone you share the following link with will be able to read this content: Get shareable link Sorry, a shareable link is not currently


available for this article. Copy to clipboard Provided by the Springer Nature SharedIt content-sharing initiative